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    北京不同背景站污染天气过程中气溶胶浓度演变及辐射效应分析

    Analysis of aerosol concentration evolution and radiative effects during pollution episodes at different background stations in Beijing

    • 摘要: 本研究探讨了不同污染天气过程中PM2.5质量浓度的日变化、小时变化特征以及气象要素、气溶胶消光系数和辐射效应的变化规律。结果表明:冬季污染过程中上甸子站PM2.5质量浓度较低且波动平缓,而南郊站PM2.5质量浓度波动较大,表现出典型的城市污染特征。秋季污染过程中上甸子站PM2.5质量浓度波动幅度略有增加,而南郊站“周末效应”减弱。上甸子站和南郊站冬季平均风速均呈下降趋势,温度上升,相对湿度增加,气象条件有利于污染物的累积;而秋季上甸子站和南郊站风速增加,表明区域输送对污染物传输起到了重要作用。冬季延庆站气溶胶消光系数整体较低,而南郊站在近地面存在明显的气溶胶消光带;秋季南郊站气溶胶消光系数在1.1 km高度较大。污染过程中气溶胶消光性的增强是导致加热率增加的主要因素。南郊站冬季气溶胶辐射加热率在近地面显著增加,而延庆站气溶胶辐射加热率较低;秋季南郊站气溶胶辐射加热率在1.1 km高度出现高值。研究结果表明,南郊站受到局地污染源和区域输送的共同影响,而延庆站主要受季节性气象条件和区域扩散的影响。为理解北京城市与郊区不同背景大气污染时空分布特征及其与气象条件的作用机制提供了科学依据。

       

      Abstract: This study investigated the diurnal and hourly variations of PM2.5 mass concentration,together with the evolution characteristics of meteorological parameters,aerosol extinction coefficients,and radiative effects during pollution episodes in different background stations in Beijing.The results show that during winter pollution episodes,PM2.5 mass concentration at Shangdianzi station were relatively low and exhibited gentle fluctuations,whereas those at the Nanjiao station exhibited substantial variability,indicating typical urban pollution characteristics.During autumn pollution episodes,the fluctuation range of PM2.5 mass concentration at Shangdianzi station increased slightly,while the "weekend effect" at Nanjiao station weakened.In winter,both Shangdianzi station and Nanjiao station exhibited a decreasing trend in wind speed accompanied by rising temperatures and increasing relative humidity,indicating meteorological conditions favorable for pollutant accumulation.In contrast,increased wind speeds at both stations during autumn indicated that regional transport played a significant role in pollutant dispersion.During winter,aerosol extinction coefficients at Yanqing station were generally low,while a distinct aerosol extinction layer was observed near the surface at Nanjiao station.During autumn,the aerosol extinction coefficients at Nanjiao station exhibited relatively high values at altitudes of 1.1 km.The enhancement of aerosol extinction during pollution episodes represented the primary factor leading to increased heating rates.In winter,aerosol radiative heating rates at Nanjiao station increased significantly near the surface,while those at Yanqing station was relatively low.In autumn,high aerosol radiative heating rates occurred around 1.1 km altitude at Nanjiao station.These results indicate that the Nanjiao station was influenced by both local emission sources and regional transport,whereas the Yanqing station was predominantly affected by seasonal meteorological conditions and regional dispersion.This study provides a scientific foundation for understanding the spatiotemporal distribution characteristics of air pollution and its interaction mechanisms with meteorological conditions at different urban and suburban background stations in Beijing.

       

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