辽宁地区O3污染状况及相关气象要素分析

doi:10.3969/j.issn.1673-503X.2021.05.005

Abstract

Abstract:

We investigated ozone pollution and related meteorological factors in Liaoning province, China using hourly surface ozone concentrations and meteorological observations for the period 2015-2019. The ozone concentrations in Liaoning province appeared to be increasing significantly in all cities, except for several cities around Liaodong Bay. Ozone has taken over PM_2.5 as the main pollutant in Liaoning province. Ozone concentrations were high in summer, but low in winter; and high in the afternoon, but low in the morning. In addition to air pollution emissions, high temperature and humidity, intense radiation, low wind speed, and air pressure were the significant meteorological factors influencing the local ozone production. With the influence of the Asian Summer Monsoon, polluted air masses from upwind direction (e. g. North China Plain) under the southwestern wind influenced the air quality over Liaoning province.

Key words: Ozone pollution, Annual variance ratio, Meteorological factor

CLC Number:

Ning-wei LIU, Wei-jun QUAN, Wan-hui REN, Xiao-lan LI, Li-guang LI, Di WANG. Ozone pollution and the related effects of meteorological factors in Liaoning province, China[J]. Journal of Meteorology and Environment, 2021, 37(5): 27-33.

Figures/Tables 10

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References 32

1	Levy II H . Normal atmosphere: large radical and formaldehyde concentrations predicted[J]. Science, 1971, 173 (3992): 141- 143. doi: 10.1126/science.173.3992.141
2	Wofsy S C , McConnell J C , McElroy M B . Atmospheric CH₄, CO, and CO₂[J]. Journal of Geophysical Research, 1972, 77 (24): 4477- 4493. doi: 10.1029/JC077i024p04477
3	IPCC. Intergovernmental panel on climate change[R]. Geneva: IPCC Secretariat, 2007.
4	Lee D S , Holland M R , Falla N . The potential impact of ozone on materials in the U.K.[J]. Atmospheric Environment, 1996, 30 (7): 1053- 1065. doi: 10.1016/1352-2310(95)00407-6
5	Danielsen E F . The laminar structure of the atmosphere and its relation to the concept of a tropopause[J]. Archiv für Meteorologie, Geophysik und Bioklimatologie, Serie A, 1959, 11 (3): 293- 332. doi: 10.1007/BF02247210
6	Reiter E R . Stratospheric-tropospheric exchange processes[J]. Reviews of Geophysics, 1975, 13 (4): 459- 474. doi: 10.1029/RG013i004p00459
7	Chameides W L , Walker J C G . A time-dependent photochemical model for ozone near the ground[J]. Journal of Geophysical Research, 1976, 81 (3): 413- 420. doi: 10.1029/JC081i003p00413
8	Logan J A . Tropospheric ozone: Seasonal behavior, trends, and anthropogenic influence[J]. Journal of Geophysical Research: Atmospheres, 1985, 90 (D6): 10463- 10482. doi: 10.1029/JD090iD06p10463
9	Ma J Z , Zhou X J , Hauglustaine D . Summertime tropospheric ozone over China simulated with a regional chemical transport model 2. Source contributions and budget[J]. Journal of Geophysical Research: Atmospheres, 2002, 107 (D22): 4612. doi: 10.1029/2001JD001355
10	刘宁微, 马建中. 东亚区域对流层臭氧及其前体物的季节性关联[J]. 应用气象学报, 2017, 28 (4): 427- 435.
11	Liu N W , Lin W L , Ma J Z , et al. Seasonal variation in surface ozone and its regional characteristics at global atmosphere watch stations in China[J]. Journal of Environmental Sciences, 2019, 77, 291- 302. doi: 10.1016/j.jes.2018.08.009
12	徐晓斌, 林伟立. 卫星观测的中国地区1979-2005年对流层臭氧变化趋势[J]. 气候变化研究进展, 2010, 6 (2): 100- 105. doi: 10.3969/j.issn.1673-1719.2010.02.005
13	Ma Z Q , Xu J , Quan W J , et al. Significant increase of surface ozone at a rural site, north of eastern China[J]. Atmospheric Chemistry and Physics, 2016, 16 (6): 3969- 3977. doi: 10.5194/acp-16-3969-2016
14	Sun L , Xue L K , Wang T , et al. Significant increase of summertime ozone at Mount Tai in Central Eastern China[J]. Atmospheric Chemistry and Physics, 2016, 16 (16): 10637- 10650. doi: 10.5194/acp-16-10637-2016
15	Xu X , Lin W , Wang T , et al. Long-term trend of surface ozone at a regional background station in eastern China 1991-2006:enhanced variability[J]. Atmospheric Chemistry and Physics, 2008, 8 (10): 2595- 2607. doi: 10.5194/acp-8-2595-2008
16	Wang T , Wei X L , Ding A J , et al. Increasing surface ozone concentrations in the background atmosphere of Southern China, 1994-2007[J]. Atmospheric Chemistry and Physics, 2009, 9 (16): 6217- 6227. doi: 10.5194/acp-9-6217-2009
17	Ding A J , Wang T , Thouret V , et al. Tropospheric ozone climatology over Beijing: analysis of aircraft data from the MOZAIC program[J]. Atmospheric Chemistry and Physics Discussions, 2007, 7 (4): 9795- 9828.
18	Wang X M , Chen F , Wu Z Y , et al. Impacts of weather conditions modified by urban expansion on surface ozone: comparison between the Pearl River Delta and Yangtze River Delta regions[J]. Advances in Atmospheric Sciences, 2009, 26 (5): 962- 972. doi: 10.1007/s00376-009-8001-2
19	Ran L , Lin W L , Deji Y Z , et al. Surface gas pollutants in Lhasa, a highland city of Tibet-current levels and pollution implications[J]. Atmospheric Chemistry and Physics, 2014, 14 (19): 10721- 10730. doi: 10.5194/acp-14-10721-2014
20	Wang Q Y , Gao R S , Cao J J , et al. Observations of high level of ozone at Qinghai Lake basin in the northeastern Qinghai-Tibetan Plateau, western China[J]. Journal of Atmospheric Chemistry, 2015, 72 (1): 19- 26. doi: 10.1007/s10874-015-9301-9
21	Yang Y , Liao H , Li J . Impacts of the East Asian summer monsoon on interannual variations of summertime surface-layer ozone concentrations over China[J]. Atmospheric Chemistry and Physics, 2014, 14 (13): 6867- 6879. doi: 10.5194/acp-14-6867-2014
22	Li X Y , Liu J F , Mauzerall D L , et al. Effects of trans-Eurasian transport of air pollutants on surface ozone concentrations over Western China[J]. Journal of Geophysical Research: Atmospheres, 2014, 119 (21): 12338- 12354. doi: 10.1002/2014JD021936
23	Li X L , Ma Y J , Wang Y F , et al. Temporal and spatial analyses of particulate matter(PM₁₀ and PM_2.5) and its relationship with meteorological parameters over an urban city in northeast China[J]. Atmospheric Research, 2017, 198, 185- 193. doi: 10.1016/j.atmosres.2017.08.023
24	刘传熙, 刘毅, 王永. 基于探空资料的北京地区大气臭氧垂直分布特征[J]. 气象与环境学报, 2016, 32 (1): 46- 52.
25	徐静. 秦皇岛市气温与近地面臭氧浓度的关系分析[J]. 气象与环境学报, 2020, 36 (4): 83- 88. doi: 10.3969/j.issn.1673-503X.2020.04.011
26	王雪松, 李金龙, 张远航, 等. 北京地区臭氧污染的来源分析[J]. 中国科学B缉: 化学, 2009, 39 (6): 548- 559.
27	余钟奇, 马井会, 毛卓成, 等. 2017年上海臭氧污染气象条件分析及臭氧污染天气分型研究[J]. 气象与环境学报, 2019, 35 (6): 46- 54. doi: 10.3969/j.issn.1673-503X.2019.06.007
28	梁碧玲, 张丽, 赖鑫, 等. 深圳市臭氧污染特征及其与气象条件的关系[J]. 气象与环境学报, 2017, 33 (1): 66- 71.
29	朱李华, 陶俊, 张仁健, 等. 冬夏季广州城区碳气溶胶特征及其与O3和气象条件的关联[J]. 环境科学学报, 2010, 30 (10): 1942- 1949.
30	国务院. 国务院关于印发大气污染防治行动计划的通知[EB/OL]. 北京: 国务院, 2013(2013-09-10)[2013-09-12]. http://www.gov.cn/zhengce/content/2013-09/13/content_4561.htm.
31	Zhang Q , Zheng Y X , Tong D , et al. Drivers of improved PM_2.5 air quality in China from 2013 to 2017[J]. Proceedings of the National Academy of Sciences of the United States of America, 2019, 116 (49): 24463- 24469.
32	张婕, 刘昊野, 辛金元, 等. 沈阳地区MODIS与MERSI气溶胶产品对比研究[J]. 遥感学报, 2016, 20 (4): 549- 560.

地点	气压	气温	相对湿度	风速	总辐射辐照度
沈阳	-0.480^*	0.413^*	-0.012	-0.016	0.352^*
大连	-0.508^*	0.509^*	0.204^*	-0.113^*	0.346^*
鞍山	-0.517^*	0.500^*	0.116^*	0.083	-
丹东	-0.022	-0.022	-0.022	-0.022	0.325^*
营口	-0.556^*	0.491^*	0.244^*	0.010	-

风向	北	北东北	东北	东东北	东	东东南	东南	南东南	南
频率/(%)	3.1	1.8	0.3	2.1	0.7	1.9	4.8	4.4	11.2

风向	南西南	西南	西西南	西	西西北	西北	北西北	静风
频率/(%)	23.9	35.1	6.5	2.3	0.3	0.3	1.0	0.3

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Ozone pollution and the related effects of meteorological factors in Liaoning province, China

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