2020年1—3月四川地区大气污染物变化特征分析

doi:10.3969/j.issn.1673-503X.2022.01.003

Abstract

Abstract:

Based on the monitoring data published by the China Environmental Monitoring Station and ground observation data of the China Meteorological Administration during 2018-2020, the variation characteristics of air pollutants in Sichuan province from January to March of 2020 were analyzed using the correlation analysis method.The results show that due to the implementation of anthropogenic emission source control policies from January to March of 2020, the concentrations of NO₂ and PM₁₀ in Chengdu, Mianyang, Yibin, and Panzhihua decrease by 30% on average compared with the same period of 2018-2019.However, the daily mean of O₃ mass concentration in the four cities increases by 15.21%, 10.32%, 5.03%, and 0.42%, respectively.At the same time, the correlation analysis of O₃ with relative humidity, temperature, wind speed, and precipitation shows that O₃ is negatively correlated with relative humidity, and positively correlated with temperature, wind speed, and precipitation, with the correlation coefficients exceeding 0.7.The abnormal growth of O₃ is not only affected by meteorological elements but also indirectly maintained by low nitrogen oxide and PM₁₀ concentrations.Strict pollutant emission control measures have a great impact on the emission of major pollutants, but less impact on secondary pollutants such as ozone.The prevention and control of secondary pollutant pollution are still facing severe challenges.

Key words: Ozone, Nitrogen dioxide, PM₁₀

CLC Number:

Wei-jie LI,Hu-jia ZHAO,Quan-liang CHEN,Lin-chang AN,Jie ZHANG,Xu-xin WANG. Variation characteristics of air pollutants in Sichuan region during January-March of 2020[J]. Journal of Meteorology and Environment, 2022, 38(1): 15-22.

Figures/Tables 6

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References 26

1	吴锴, 康平, 王占山, 等. 成都市臭氧污染特征及气象成因研究[J]. 环境科学学报, 2017, 37 (11): 4241- 4252.
2	柯伯俊. 四川省大气污染源排放清单研究[D]. 西南交通大学, 2014.
3	周书华, 倪长健, 刘培川. 成都地区大气边界层逆温特征分析[J]. 气象与环境学报, 2015, 31 (2): 108- 111.
4	周启星. 气候变化对环境与健康影响研究进展[J]. 气象与环境学报, 2006, 22 (1): 38- 44. doi: 10.3969/j.issn.1673-503X.2006.01.009
5	刘华悦, 付桂琴, 王洁. 石家庄市气象要素对成人哮喘住院人数的影响[J]. 气象与环境学报, 2019, 35 (5): 137- 143. doi: 10.3969/j.issn.1673-503X.2019.05.018
6	Nuvolone D , Petri D , Voller F . The effects of ozone on human health[J]. Environmental Science and Pollution Research International, 2018, 25 (9): 8074- 8088. doi: 10.1007/s11356-017-9239-3
7	Seinfeld J H , Pandis S N . From air pollution to climate change[J]. Atmospheric Chemistry and Physics, 1998, 1326
8	杨昆, 黄一彦, 石峰, 等. 美日臭氧污染问题及治理经验借鉴研究[J]. 中国环境管理, 2018, 10 (02): 85- 90.
9	Paoletti E , Marco A D , Beddows D C S , et al. Ozone levels in European and USA cities are increasing more than at rural sites, while peak values are decreasing[J]. Environmental Pollution, 2014, 192 (9): 295- 299.
10	Lefohn A S , Malley C S , Smith L , et al. Tropospheric ozone assessment report: global ozone metrics for climate change, human health, and crop/ecosystem research[J]. Elementa(Washington, D.C.), 2018, 1, 1.
11	Lauri Myllyvirta . 蓝天保卫战: 能源行业的下一个挑战在哪里?[J]. 能源, 2020, (Z1): 29- 30.
12	Karl T , Graus M , Striednig M , et al. Urban eddy covariance measurements reveal significant missing NOx emissions in Central Europe[J]. Entific Reports, 2017, 7 (1): 13849- 13893.
13	Monks P S , Archibald A T , Colette A , et al. Tropospheric ozone and its precursors from the urban to the global scale from air quality to short-lived climate forcer[J]. Atmospheric Chemistry and Physics, 2015, 15, 8889- 8973. doi: 10.5194/acp-15-8889-2015
14	郝吉明, 田贺忠. 中国氮氧化物排放现状、趋势及控制对策建议[C]. //2004全国燃煤二氧化硫、氮氧化物污染治理技术研讨会技术汇编. 中国环境科学学会, 2004: 362-371.
15	Huang K , Zhuang G , Lin Y , et al. Impact of anthropogenic emission on air quality over a megacity-revealed from an intensive atmospheric campaign during the Chinese spring festival[J]. Atmospheric Chemistry and Physics, 2012, 12 (23): 11631- 11645. doi: 10.5194/acp-12-11631-2012
16	周子航, 邓也, 谭钦文, 等. 四川省人为源大气污染物排放清单及特征[J]. 环境科学, 2018, 39 (12): 5344- 5358.
17	徐晨曦, 陈军辉, 李媛, 等. 四川省基于第二次污染源普查数据的人为源大气污染源排放清单及特征[J/OL]. 环境科学: 1-18[2020-07-14]. https://doi.org/10.13227/j.hjkx.202002162.
18	Sicard P , De Marco A , Agathokleous E , et al. Amplified ozone pollution in cities during the COVID-19 lockdown[J]. Science of The Total Environment, 2020, 735, 139542. doi: 10.1016/j.scitotenv.2020.139542
19	郑丽英, 许婷婷, 陈志安, 等. 成都市夏季臭氧污染特征及影响因素[J]. 气象与环境学报, 2019, 35 (5): 78- 84. doi: 10.3969/j.issn.1673-503X.2019.05.010
20	He Z , Wang X , Ling Z , et al. Contributions of different anthropogenic volatile organic compound sources to ozone formation at a receptor site in the Pearl River Delta region and its policy implications[J]. Atmospheric Chemistry and Physics, 2019, 19 (13): 8801- 8816. doi: 10.5194/acp-19-8801-2019
21	Chen Z , Li R , Chen D , et al. Understanding the causal influence of major meteorological factors on ground ozone concentrations across China[J]. Journal of Cleaner Production, 2020, 242, 118498. doi: 10.1016/j.jclepro.2019.118498
22	Solberg S , Bergstroem R , Langner J , et al. Changes in Nordic surface ozone episodes due to European emission reductions in the 1990s[J]. Atmospheric Environment, 2005, 39 (1): 179- 192. doi: 10.1016/j.atmosenv.2004.08.049
23	Pierre Sicard , Romain Serra , Philippe Rossello . Spatiotemporal trends in ground-level ozone concentrations and metrics in France over the time period 1999-2012[J]. Environmental Research, 2016, 149 (aug.): 122- 144.
24	Li M , Wang T , Xie M , et al. Impacts of aerosol-radiation feedback on local air quality during a severe haze episode in Nanjing megacity, eastern China[J]. Tellus B: Chemical and Physical Meteorology, 2017, 69 (1): 1339548. doi: 10.1080/16000889.2017.1339548
25	Wolff G T , Kahlbaum D F , Heuss J M . The vanishing ozone weekday/weekend effect[J]. Journal of the Air & Waste Management Association, 2013, 63 (3): 292- 299.
26	Li J , Wang Z , Wang X , et al. Impacts of aerosols on summertime tropospheric photolysis frequencies and photochemistry over Central Eastern China[J]. Atmospheric Environment, 2011, 45 (10): 1817- 1829. doi: 10.1016/j.atmosenv.2011.01.016

要素	1月	2月	3月
最大值/(μg·m^-3)	68.71	70.34	74.37
平均值/(μg·m^-3)	25.51	47.13	46.99
累积超标天数/d	0	0	0

气象要素	NO₂	O₃	PM₁₀	1月	2月	3月
相对湿度	0.21	-0.71	0.08	4.68%	-4.56%	-4.86%
温度	0.11	0.88	-0.09	15.43%	25.69%	8.33%
风速	-0.25	0.72	-0.48	-6.58%	10.25%	6.18%
降水	0.09	0.66	-0.22	15.61%	12.20%	-28.57%

城市	气象要素	相关系数	显著性	相关性
绵阳	相对湿度	- 0.72	0.030	负相关
	温度	0.92	0.001	正相关
	风速	0.77	0.016	正相关
	降水	0.71	0.032	正相关
宜宾	相对湿度	- 0.80	0.010	负相关
	温度	0.96	0.000	正相关
	风速	0.79	0.012	正相关
	降水	0.20	0.600	正相关
攀枝花	相对湿度	- 0.90	0.001	负相关
	温度	0.87	0.003	正相关
	风速	0.71	0.032	正相关
	降水	-0.65	0.059	负相关

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[15]	JIANG Lu-lu, QIAN Yan-zhen, DU Kun, GU Xiao-li. Variation of ozone concentration and prediction in surface layer in Ningbo [J]. Journal of Meteorology and Environment, 2016, 32(1): 53-59.

Variation characteristics of air pollutants in Sichuan region during January-March of 2020

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